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Often compared to Rex Harrison, Mulhare had his two greatest US successes inheriting roles that Harrison created. On Broadway, Mulhare succeeded Harrison as Henry Higgins in "My Fair Lady" when the latter joined the London company, playing the part for most of the play's remaining Broadway run. On television, Mulhare played the role of the ghost of Captain Daniel Gregg in the TV version of "The Ghost and Mrs. Muir", a role Harrison had created two decades earlier in the film version.